:v Depends on your bore diameter, the .610" ball may require a veerry thin patch as most .62's seem to have a .610" bore. If the .610 work for you, I do have a mold for .610Rb that I'd gladly give you a great deal on.
I have a 62 cal underhammer rifle that the builder furnished with a .610 mold, this required a .005-.010 patch. Terrible time with burning/torn patches until this spring. Completed a 62 smoothbore with a .610 bore, so I got a .600"mold, the smoothie shoots great with the .600, tried it in the 62 rfle with a .015-.020" patch now the rifle shoots better than ever with less powder for the same velocity and no burnt patches. Fit is almost everything.
Try some harder .600 balls as they will not swage in the barrel and remain round, this is important in flight at longer distances. A round ball with cylinderical sides will really start to wander beyond 50 yards or so. :v