The .456” 220 grain molds have solved a number of problems for me, but I only run straight lead or 40:1 alloy, and use sizing dies to fine tune the diameter that works.
Though I’ve not tried casting with bismuth (I have more than enough irons in the fire), I have to wonder how long a Lee aluminum mold would hold up casting it? But it sounds like it may be worth trying if you can knurl the bismuth diameter up. I use a knurling attachment from lathe and find I can increase the OD on copper .005” to .008”, depending on the alloy and my determination.