Yup, start in the 60-70 grain neighborhood and work up. I kinda work "backwards" based on my needs for trajectory and experience with 54 cal. I start at 80 grains, with 2f and then 3f black, then go up to 90. If I'm not getting the accuracy I want I'll go up to 100. Still not getting the accuracy? I'll usually drop down to 70 then, but with disappointment. I don't need higher than 100 for my shooting, but by the time I get down to 70 my trajectory is starting to suffer. Most of my 54's like 90 grains of one granulation or the other. I'm currently using 90 grains of 3f Goex in my GPR 54.
My hunting pard is the 777 user in our crowd. His particular rifle just sings with 90 grains of 777 in 3f granulation. That's the rough equivalent of 100-105 grains of 3f Goex, but his rifle likes what it likes.
One thing to watch with yours is patch condition. With that .535 ball you might find .015 patches a little hard to load if you haven't shot that gun at least a couple of hundred times in the past, and you'll be tempted to go to .010 patches to ease loading. In my experience, that's almost a sure formula for torn patches and poor accuracy. Better would be to go to a .530 ball and .015 or .018 patches in that case. But don't complicate things unnecessarily. Go ahead and shoot what you have, then start changing ball/patch if you're getting torn patches.